I would try to check RAM chips 512KB at a time, maybe one of your RAM chips are bad. Set the jumper to 512KB, start the computer and see it it works, if it does then try 1MB, you can try with the chips inserted or remove them all and try 512KB at a time.
Also, do you have any other RAM board installed?
Yep, did that... it did the same thing at 512K, and 1MB. The only jumper that apparently works is 0MB.
No other add on cards; it's a stock A2000 with just the A2091.
I had three A2000's given to me, and I've been working through them to get some workable systems. So far, I have:
A2000 (stock 512K chip/512K fast) with A2091, unknown (haven't checked) SCSI drive, WB 2.04. One floppy drive; inoperative. Front cover has three screw stands broken on it; I need to see if I can epoxy them back. Someone hacked the PSU and cut off one of the Molex connectors. Has an additional SCSI drive that came with it, but it wasn't hooked up. Haven't tried it yet. No keyboard/mouse.
A2000 (has 2MB chip ram mod) with GVP 68030 (33mhz?) accelerator/SCSI and 16MB RAM card installed with 3.5" SCSI hard drive in bottom bay. Two floppy drives; both inoperative. PSU good, case is good, need to get additional screws for it. Cleaned up the case (scrubbed it real good), so the only real problem with this one is it needs new floppies and some screws. Keyboard and mouse.
A2000 (has 2MB chip ram mod) with 68040/25 accelerator/SCSI and a crapload of RAM (haven't done an avail on it yet) with attached 3.5" SCSI hard drive on the back of the accelerator. Has flicker fixer in video slot with VGA connector. Also has a PVR card (records video, encodes with JPG/MPG?). PSU good, case is good, have all the screws. Cleaned up the case. One floppy drive, seems to work OK, but was touchy until I cleaned it. Keyboard with Toaster stickers on it and mouse. Intermittently booted up with green screen, but I reseated Agnus and the pin that went to Gary (I think) and it is happy again.
Also have six TBC cards, five with passthroughs, and a Video Toaster 2000.
I probably will keep the 68040 system but the rest will be fair game. If I six the floppy drive issues by getting refurbs from Software Hut, I'll just tack it onto the price (one I'm probably giving away, the other two likely will be sold), or let whomever is going to be getting this buy the replacement and swap it out. I hooked an external floppy up to make sure the floppy controller was working on all three.

There was lots of dirt, grime, cigarette smoke, etc, on these, so it's been a labor of love fixing them up.