I agree completely and understand the risks. 66mhz was as high as I was willing to go, will probably settle at 55 or maybe even 60
I understand the desire to squeeze more out of your machine but I would advise against, to be honest. Back in the day, I overclocked my old 68040 from 25 to 30MHz (equivalent to your proposed 50 -> 60 MHz). It didn't make a huge difference in terms of performance to be fair and was less stable.
Now I look at it from the point of view of longevity. I'd much rather have a stable system than a slightly faster one.
If I want raw speed for 68K apps, I use UAE. It's pretty much impossible to beat.